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Das Ziel dieser Arbeit ist es, zu untersuchen, ob Ionische Flüssigkeiten eine neuartige Metalcarbonyl Chemie ermöglichen. Die Reaktivität von Metallcarbonylen in imidazoliumbasierten Ionischen Flüssigkeiten wurde untersucht. Dabei konnte eine Anzahl neuartiger Metallcarbonyl-, Koordinations und Netzwerkverbindungen realisiert werden: [BMIm]6[S][{Fe(CO)3}4(SnI)6I4]2, [BMIm]2[{Fe(CO)3}4(SnI)6I4], [AIm][FeI(CO)3(SnI3)2] (AIm: EMIm, EHIm, PMIm), Te2Fe(CO)4{Fe(CO)3}2, [BMIm][{Te2}3{Mn(CO)3}2{Mn(CO)4}3], [BMIm][M(OTf)3], (M: Fe, Mn), [AIm][Li(OTf)2] (AIm: BMIm, EMIm), [EMIm][{GeI4}2I], [Co{1,4-(CN)2C6H4}2(NTf2)2][SnI(Co(CO)4)3]2, CoI2{1,3-(CN)2C6H4} und FeI2{1,4-(CN)2C6H4}.