Introduction.- Regioselective Insertion of -Carborynes into -C-H Bond of Tertiary Amines.- Synthesis of Carborane-Functionalized Heterocycles: Dearomative [2 + 2] Cycloaddition and sp2 C-H Insertion Reaction.- Reaction of -Carboryne with Nitrones: A Formal [5 + 2] Cycloaddition.- 1,3-Dehydro--Carborane: Generation and Reaction with Arenes.- Ene Reaction of 1,3-Dehydro--Carborane.- Cage Boron Arylation of -Carborane via Metal-Free, Visible-Light-Mediated Radical Coupling.- Conclusion.- Experimental Section.
Introduction.- Regioselective Insertion of -Carborynes into -C-H Bond of Tertiary Amines.- Synthesis of Carborane-Functionalized Heterocycles: Dearomative [2 + 2] Cycloaddition and sp2 C-H Insertion Reaction.- Reaction of -Carboryne with Nitrones: A Formal [5 + 2] Cycloaddition.- 1,3-Dehydro--Carborane: Generation and Reaction with Arenes.- Ene Reaction of 1,3-Dehydro--Carborane.- Cage Boron Arylation of -Carborane via Metal-Free, Visible-Light-Mediated Radical Coupling.- Conclusion.- Experimental Section.
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