Despite major advances and a wide range of interest in the field across chemistry, the medical sciences and biophysics, there have been very few up-to-date books on the subject. Bringing together the latest information and advances on this topic, this book provides a broad, yet detailed view of both theory and applications. Die Übertragung elektronischer Energie zwischen Molekülen oder verschiedenen Positionen desselben Moleküls spielt eine wichtige Rolle in der modernen Chemie, der Medizin und der Biophysik. Bisher gab es kein Buch, das Grundprinzipien und Anwendungen dieses Gebietes…mehr
Despite major advances and a wide range of interest in the field across chemistry, the medical sciences and biophysics, there have been very few up-to-date books on the subject. Bringing together the latest information and advances on this topic, this book provides a broad, yet detailed view of both theory and applications.Die Übertragung elektronischer Energie zwischen Molekülen oder verschiedenen Positionen desselben Moleküls spielt eine wichtige Rolle in der modernen Chemie, der Medizin und der Biophysik. Bisher gab es kein Buch, das Grundprinzipien und Anwendungen dieses Gebietes gleichermaßen umfassend behandelte - eine Lücke, die jetzt geschlossen ist. Theoretische, mechanistische und praxisbezogene Aspekte kommen gleichermaßen zur Sprache. (04/99)
David L. Andrews, School of Chemical Sciences, University of East Anglia, GB. Highly respected and has made major interesting contributions in the field. His works are very deep and illuminating. Professor Andrews has also published in condensed matter QED, though not to the same extent. One of his books has gone to a third edition, and another has been reprinted.
Inhaltsangabe
1. Resonance energy transfer in proteins introduction some basic considerations a short history of FRET determinations the components of the Foorster equation quantum yield determining spectral overlap steady state or time-resolved measurements? resonance energy transfer using intrinsic amino acids homotransfer between intrinsic probes heterotransfer the range of distances determined by resonance energy transfer precise location of resonance energy transfer probes properties of probes labeling specific residues in proteins resonance energy transfer experiments using lanthanide ions measurements in radially symmetrical systems comparison with crystallographic distances using resonance energy transfer to constrain molecular models resonance energy transfer with single fluorophores: new wave experiments intramolecular energy transfer in proteins bound to membranes green fluorescent protein resonance energy transfer and biosensors: a new and promising technique shortcomings the future of FRET summary dedication acknowledgements references. 2. Unified theory and radiative and raditionless energy transfer introduction background the basis of the unified theory spectral features refraction and dissipation dynamics of energy transfer between a pair of molecules in a dielectric medium conclusion appendix A: Heitler-MA method for analysis of the transition operator Appendix B: modified approach to the transition operator references. 3. Dynamics of radiative transport introduction overview of atomic and molecular radiative transport the Holstein-Biberman equation multiple scattering representation stochastic approach combined radiative and nonradiative transport conclusion appendix A: probablitity of emission of a photon between t + dt for an nth generation molecule appendix B: depolarization factor for radiative transferaccording to classical electrodynamics references. 4. Orientational aspects in pair energy transfer introduction Kappa-squared and probability, Kappa-squared and anisotropy notes on the effects of order and motion acknowledgements references. 5. Polarization in molecular complexes with incoherent energy transfer introduction interaction of light with single molecules or chromophores bichromophore molecular complexes trichromophore complexes multichromophore complexes with C3 symmetry conclusion appendix A appendix B appendix C appendix D references. 6. Theory of coupling in multichromophoric systems introduction reactant and product states: LMO model the origin of coupling matrix elements paradigmatic results coulombic coupling superexchange interpretation of steady state spectra calculation of couplings acknowledgements references. 7. Exciton annihilation in molecular aggregates introduction theory applications discussion acknowledgements references. 8. Energy transfer and localization: applications to photosynthetic systems introduction optical properties of dimers and aggregates energy and localization in antenna complexes and reaction centers acknowledgements references. 9.Excitation energy transfer in photosynthesis introduction the structure of light-harvesting complexes the mechanism of energy transfer and trapping in photosynthesis dynamics of excitation energy transfer conclusions acknowledgements references. 10. The Fenna-Matthews-Olson protein: a strongly coupled photosynthetic antenna introduction steady state spectroscopy FMO exciton simulations FMO primary processes epilog and future prospects acknowledgements references. 11. Use of a Monte carlo method in the problem of energy migration in molecular complexes introduction an illustration of Monte Carlo calculations in the problem of fluorescence decay energy transfer in CME: major algorithm applications of monte Carlo simulations conclusion acknowledgements references. Index
1. Resonance energy transfer in proteins introduction some basic considerations a short history of FRET determinations the components of the Foorster equation quantum yield determining spectral overlap steady state or time-resolved measurements? resonance energy transfer using intrinsic amino acids homotransfer between intrinsic probes heterotransfer the range of distances determined by resonance energy transfer precise location of resonance energy transfer probes properties of probes labeling specific residues in proteins resonance energy transfer experiments using lanthanide ions measurements in radially symmetrical systems comparison with crystallographic distances using resonance energy transfer to constrain molecular models resonance energy transfer with single fluorophores: new wave experiments intramolecular energy transfer in proteins bound to membranes green fluorescent protein resonance energy transfer and biosensors: a new and promising technique shortcomings the future of FRET summary dedication acknowledgements references. 2. Unified theory and radiative and raditionless energy transfer introduction background the basis of the unified theory spectral features refraction and dissipation dynamics of energy transfer between a pair of molecules in a dielectric medium conclusion appendix A: Heitler-MA method for analysis of the transition operator Appendix B: modified approach to the transition operator references. 3. Dynamics of radiative transport introduction overview of atomic and molecular radiative transport the Holstein-Biberman equation multiple scattering representation stochastic approach combined radiative and nonradiative transport conclusion appendix A: probablitity of emission of a photon between t + dt for an nth generation molecule appendix B: depolarization factor for radiative transferaccording to classical electrodynamics references. 4. Orientational aspects in pair energy transfer introduction Kappa-squared and probability, Kappa-squared and anisotropy notes on the effects of order and motion acknowledgements references. 5. Polarization in molecular complexes with incoherent energy transfer introduction interaction of light with single molecules or chromophores bichromophore molecular complexes trichromophore complexes multichromophore complexes with C3 symmetry conclusion appendix A appendix B appendix C appendix D references. 6. Theory of coupling in multichromophoric systems introduction reactant and product states: LMO model the origin of coupling matrix elements paradigmatic results coulombic coupling superexchange interpretation of steady state spectra calculation of couplings acknowledgements references. 7. Exciton annihilation in molecular aggregates introduction theory applications discussion acknowledgements references. 8. Energy transfer and localization: applications to photosynthetic systems introduction optical properties of dimers and aggregates energy and localization in antenna complexes and reaction centers acknowledgements references. 9.Excitation energy transfer in photosynthesis introduction the structure of light-harvesting complexes the mechanism of energy transfer and trapping in photosynthesis dynamics of excitation energy transfer conclusions acknowledgements references. 10. The Fenna-Matthews-Olson protein: a strongly coupled photosynthetic antenna introduction steady state spectroscopy FMO exciton simulations FMO primary processes epilog and future prospects acknowledgements references. 11. Use of a Monte carlo method in the problem of energy migration in molecular complexes introduction an illustration of Monte Carlo calculations in the problem of fluorescence decay energy transfer in CME: major algorithm applications of monte Carlo simulations conclusion acknowledgements references. Index
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