Metalloenzymes as Inspirational Electrocatalysts for Artificial Photosynthesis

Metalloenzymes as Inspirational Electrocatalysts for Artificial Photosynthesis

From Mechanism to Model Devices

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This thesis describes a series of investigations designed to assess the value of metalloenzymes in systems for artificial and adapted photosynthesis. The research presented explores the interplay between inherent enzyme properties such as structure, rates and thermodynamics, and the properties of the semiconducting materials to which the enzyme is attached. Author, Andreas Bachmeier provides a comprehensive introduction to the interdisciplinary field of artificial photosynthesis, allowing the reader to grasp the latest approaches being investigated, from molecular systems to heterogeneous surf...