Cindy Wechsler
Broschiertes Buch

Intermediates in the carboligation of the ThDP-dependent pyruvate decarboxylase. Tailor-made enzyme catalysts for industrial applications

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As enzymatic transformations become more and more recognized as practical alternative for synthetic applications, one objective of this thesis was to contribute to the industrial synthetic portfolio with newly designed tailor-made catalysts. The main objective however was to perform a comprehensive study on the prototypical ThDP-dependent enzyme pyruvate decarboxylase to deduce mechanistic principles by which the fate of reaction intermediates are conferred. Within this thesis, mechanistic studies on pyruvate decarboxylase from Z. mobilis have been performed with relevance for asymmetric carbo...