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Thesis submitted to the faculty of the Graduate School of the University of Minnesota in partial fulfillment of the requirements for the degree of Doctor of Philosophy. Part I discusses the spatial correlation between the x-ray and radio morphologies of Cas A, and in the process address: the effect of inhomogeneous absorption on the apparent x-ray morphology, the interaction between the SNR and a molecular cloud, and the rapid move toward equipartition between the magnetic and gas energy densities. Discussions of the x-ray./radio correlation continues in Chapter 5, where we present a new, deep, ROSAT HRI image of Cas A. Chapter 7 presents ASCA spectra, with non-thermal spectral fits for 13 of the youngest SNRs in the Galaxy.