René Costard
eBook, PDF

Ultrafast Dynamics of Phospholipid-Water Interfaces (eBook, PDF)

Studied by Nonlinear Time-Resolved Vibrational Spectroscopy

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This thesis presents a highly innovative study of the ultrafast structural and vibrational dynamics of hydrated phospholipids, the basic constituents of cell membranes. As a novel approach to the water-phospholipid interface, the author studies phosphate vibrations using the most advanced methods of nonlinear vibrational spectroscopy, including femtosecond two-dimensional infrared spectroscopy. He shows for the first time that the structure of interfacial water undergoes very limited fluctuations on a 300 fs time scale and that the lifetimes of hydrogen bonds with the phospholipid are typicall...

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