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Proton Exchange Membrane Fuel Cells Platinum-Free Oxygen Reduction and Performance Degradation by Start-Up/Shut-Down Events (eBook, PDF)

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Two major hindrances prevent proton exchange membrane fuel cells (PEMFCs) from being of widespread commercial success: high costs and limited durability. One of the main cost contributors is platinum which is currently used in the catalyst layers, mainly for the oxygen reduction reaction. This work aims for a comprehensive understanding of the oxygen reduction electrocatalysis associated with two specific platinum-free materials, palladium and completely noble-metal-free transition metal oxides. Among other lifetime limiting factors, the transient operation state of start-up and/or...

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