Singlet Delta Oxygen: A Quantitative Analysis Using Off-Axis Integrated-Cavity-Output-Spectroscopy
Jeffrey E. Gallagher
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Singlet Delta Oxygen: A Quantitative Analysis Using Off-Axis Integrated-Cavity-Output-Spectroscopy

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A new spectroscopic technique applicable to the detection of ultra-weak and for- bidden molecular transitions is presented. The method is based on o -axis integrated- cavity-output spectroscopy (ICOS) and has been applied to the detection of singlet (a1 g) oxygen in the (1,0) band of the electric-quadrupole allowed Noxon system (b1 + g a1 g) of oxygen. The details of the method as well as spectroscopic data con rming the absolute line positions of twenty-one lines in the (1,0) band of the b1 + g a1 g have been completed to within 0:004 cm 1. A Boltzmann analysis veri ed previously calculated a...