Dissociative Recombination
Theory, Experiment, and Applications
Herausgegeben von Rowe, Bertrand R.; Mitchell, J. Brian A.; Canosa, André
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InMay1988,theFirstInternationalConferenceonDissociativeRecombination:Theory, ExperimentandApplicationswasheldatChateauLakeLouise,Alberta,Canada. Thismeeting gaveaconsiderableimpetustothissubject,whichisofparticularinterestforalargevarietyof fieldsincludinginterstellarclouds,planetaryatmospheres,gaslasers,plasmaprocessing,ion sourcesandthermonuclearplasmas. Sincethen,indeed,severalcollaborationswereinitiated betweenexperimentalistsworkingwithdifferenttechniques,betweentheoreticiansdealingwith molecularstructureononehandanddynamicsontheotherhandandalsobetween experimentalistsandtheoreticians. Du...
InMay1988,theFirstInternationalConferenceonDissociativeRecombination:Theory, ExperimentandApplicationswasheldatChateauLakeLouise,Alberta,Canada. Thismeeting gaveaconsiderableimpetustothissubject,whichisofparticularinterestforalargevarietyof fieldsincludinginterstellarclouds,planetaryatmospheres,gaslasers,plasmaprocessing,ion sourcesandthermonuclearplasmas. Sincethen,indeed,severalcollaborationswereinitiated betweenexperimentalistsworkingwithdifferenttechniques,betweentheoreticiansdealingwith molecularstructureononehandanddynamicsontheotherhandandalsobetween experimentalistsandtheoreticians. Duringthelastfouryears,therefore,alargenumberof studieswerecarriedoutandraisedanewsetofquestions. Moreparticularly,theresultsthat wereobtainedconcerningcontroversialspeciessuchasH!andHeir,castingsomedoubton theverymechanismsbywhichdissociativerecombinationproceeds. The Second International Conference on Dissociative Recombination: Theory, ExperimentandApplications heldat"I'AbbayedeSaintJacutdelaMer",Brittany,France, May3-8,1992,camethereforeattherighttimetosurveythecurrentstateofthesubject. The symposiumbroughttogetherleadinginvestigatorsinthefieldsofmolecularionrecombination research,atomicandmoleculartheoryandexperiment,plasmasphysics,astrochemistryand aeronomy. Speakerspresentedtalksreviewingtheirownworkandthesewerefollowedby livelydiscussionsessions. Freetimeperiodsallowedparticipantstodiscoveranenchanting peninsulaofNorthBrittanywhilepursuingstimulatingscientificdiscussions. Thepapersinthis volumearebasedonthesetalksandfurtherdiscussions,withtheexceptionofcontributions fromT. AmanoandB. M. McLaughlinwhowereunabletoattend. Alistofparticipantsas wellasasouvenirgroupphotoisgivenattheendofthebook. WeareindebtedtoNATOforitsfinancialsupportwhichcontributedtothegreat successofthissecondmeeting. TheUniversityofRennesIandtheBalzerscompanyarealso acknowledgedfortheiradditionalsupportManythankstothewholestaffoftheabbeyforits kindnessandeffortsinprovidinguswithapropitiousenvironmentforsuchaworkshop. We arealsogratefultoL. Caubetforhervaluableadministrativeassistanceduringthepreparation ofthemeeting. Finallyaspecialmentionmustbegiventoallthesessionchairpersonsfortheir skillinorchestratingthediscussions. Lookingforwardtoattendingthethirdmeeting. TheEditors Bertrand R. Rowe J. Bria/l A. Mitchell Andre Callosa DepartementdePhysique DepartmentofPhysics DepartementdePhysique AtomiqueetMoleculaire TheUniversityofWesternOntario AtomiqueetMoleculaire UniversitedeRennesI London,Canada,N6A3K7 UniversitedeRennesI CampusdeBeaulieu CampusdeBeaulieu 35042RennesCedex, 35042RennesCedex, France France v CONTENTS ORALCONTRIBUTIONS PolyatomicIonDissociativeRecombination . 1 D. R. Bates RecentDevelopmentsandPerspectivesintheTreatmentofDissociative RecombinationandRelatedProcesses. . . . . . . . . . . . . . . . . . . . . . . . . . . 11 A. Giusti-Suzor, I. F Schneider, and 0. Dulieu CharacteristicsofSuperexcitedStatesofMoleculesandMQDTStudiesofNO+ DissociativeRecombination. . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . 25 H. Sun, K. Nakashima, and H. Nakamura CalculationsforAr +Xe andArXe+ +e 35 A. P. Hickman, DL Huestis, and R. P. Saxon Electron-IonContinuum-ContinuumMixinginDissociativeRecombination 47 s. L. Guberman ATheoreticalStudyoftheHCO+andHCS+ElectronicDissociativeRecombinations. . 59 D. Talbi, and Y Ellinger DissociativeRecombinationofCH;:SomeBasicInformationfromElectronic 2 StructureCalculations. 67 WP. Kraemer TheoreticalProblemsintheDissociativeRecombinationofH~ +e. . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . 75 H. Takagi RecentMergedBeamsInvestigationsofHydrogenMolecularIonRecombination. . . . . . . 87 J B. A. Mitchell, F B. Yousif, P. Van der Donk, and T. J Morgan vii FlowingAfterglowStudiesofElectron-IonRecombinationusingLangmuirProbesand OpticalSpectroscopy. . . . . . . 99 NG. Adams RecentFlowingAfterglowMeasurements . 113 B. R. Rowe
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